DS2Key Sypherce has released a very handy application for the Nintendo DS, DS2Key v0.11. DS2Key sends PC keyboard signals through WiFi so that you can use your DS somewhat like a PC gamepad. In essence, you can use the DS as a controller to contorl emulated games on your PSP. Set up directions are included in the readme file.
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MythRemote PC owners with the MythTV home entertainment app hooked up may want to take a gander
KnobsandSlidersDS-0.3 This software allows you to use your Nintendo DS touchscreen to control things remotely over wifi